So the current behavior of Mastodon is if you click the boost button it offers a popup box asking if you want to boost or quote-boost, and if you hold shift and click the boost button it boosts. I have no current plans to ever quote boost because that does not match how I use this website. I wonder if I could reverse that behavior. Click to boost, shift-click to get the unusual menu w/quote boost.

This isn't an option, right? Could I use Tampermonkey?

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If you have a fediverse account, you can quote this note from your own instance. Search https://mastodon.social/users/mcc/statuses/115226034792369850 on your instance and quote it. (Note that quoting is not supported in Mastodon.)